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Peer-reviewed

Source Apportionment of Atmospheric Ammonia at 16 Sites in China Using a Bayesian Isotope Mixing Model Based on δ<sup>15</sup>N–NH<sub><i>x</i></sub> Signatures

Yangyang Zhang, Xin Ma, Aohan Tang, Yunting Fang, T. H. Misselbrook, Xuejun Liu

Environmental Science & Technology · 2023

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Summary

Reducing atmospheric ammonia (NH<sub>3</sub>) emissions is critical to mitigating poor air quality. However, the contributions of major agricultural and non-agricultural source emissions to NH<sub>3</sub> at receptor sites remain uncertain in many regions, hindering the assessment and implementation of effective NH<sub>3</sub> reduction strategies. This study conducted simultaneous measurements of the monthly concentrations and stable nitrogen isotopes of NH<sub><i>x</i></sub> (gaseous NH<sub>3</sub> plus particulate NH<sub>4</sub><sup>+</sup>) at 16 sites across China. Ambient NH<sub><i>x</i></sub> concentrations averaged 21.7 ± 19.6 μg m<sup>-3</sup> at rural sites, slightly higher than those at urban (19.2 ± 6.0 μg m<sup>-3</sup>) and three times of those at background (7.0 ± 6.9 μg m<s

Source type
Peer-reviewed study
DOI
10.1021/acs.est.2c09796
Catalogue ID
SNmoef2b63-opt5bp
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