Pulse Brain · Growing Health Evidence Index
Peer-reviewed

Soil Emissions of Reactive Nitrogen Accelerate Summertime Surface Ozone Increases in the North China Plain

Wanshan Tan, Haolin Wang, Jiayin Su, Ruize Sun, Cheng He, Xiao Lu, Jintai Lin, Chaoyang Xue, Haichao Wang, Yiming Liu, Lei Liu, Lin Zhang, Dianming Wu, Yujing Mu, Shaojia Fan

Environmental Science & Technology · 2023

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Summary

Summertime surface ozone in China has been increasing since 2013 despite the policy-driven reduction in fuel combustion emissions of nitrogen oxides (NO<sub><i>x</i></sub>). Here we examine the role of soil reactive nitrogen (N<sub>r</sub>, including NO<sub><i>x</i></sub> and nitrous acid (HONO)) emissions in the 2013-2019 ozone increase over the North China Plain (NCP), using GEOS-Chem chemical transport model simulations. We update soil NO<sub><i>x</i></sub> emissions and add soil HONO emissions in GEOS-Chem based on observation-constrained parametrization schemes. The model estimates significant daily maximum 8 h average (MDA8) ozone enhancement from soil N<sub>r</sub> emissions of 8.0 ppbv over the NCP and 5.5 ppbv over China in June-July 2019. We identify a strong competing effect bet

Source type
Peer-reviewed study
DOI
10.1021/acs.est.3c01823
Catalogue ID
SNmoht1xk5-3yt4eb
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